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Most collections I am aware of are worth more if you piece them out, unless it is a comprehensive and complete set of something. A hodge-podge of items, like ammunition, probably could not fit in this category since there are so many obscure rounds, some of which I'm sure only a handful were ever made.
You could probably piece it out and make more on it, but that would be tedious and take forever and in the end you would be left with a number of cartridges that might not be worth anything, but you don't want to throw away.
I would sell it as a lot if I were you.